Estimation of Potentially Toxic Elements Contamination in Anthropogenic Soils on a Brown Coal Mining Dumpsite by Reflectance Spectroscopy: A Case Study
Identifieur interne : 000091 ( Main/Exploration ); précédent : 000090; suivant : 000092Estimation of Potentially Toxic Elements Contamination in Anthropogenic Soils on a Brown Coal Mining Dumpsite by Reflectance Spectroscopy: A Case Study
Auteurs : Asa Gholizadeh [République tchèque] ; Luboš Borůvka [République tchèque] ; Radim Vašát [République tchèque] ; Mohammadmehdi Saberioon [République tchèque] ; Aleš Klement [République tchèque] ; Josef Kratina [République tchèque] ; Václav Tejneck [République tchèque] ; Ond Ej Drábek [République tchèque]Source :
- PLoS ONE [ 1932-6203 ] ; 2015.
Abstract
In order to monitor Potentially Toxic Elements (PTEs) in anthropogenic soils on brown coal mining dumpsites, a large number of samples and cumbersome, time-consuming laboratory measurements are required. Due to its rapidity, convenience and accuracy, reflectance spectroscopy within the Visible-Near Infrared (Vis-NIR) region has been used to predict soil constituents. This study evaluated the suitability of Vis-NIR (350–2500 nm) reflectance spectroscopy for predicting PTEs concentration, using samples collected on large brown coal mining dumpsites in the Czech Republic. Partial Least Square Regression (PLSR) and Support Vector Machine Regression (SVMR) with cross-validation were used to relate PTEs data to the reflectance spectral data by applying different preprocessing strategies. According to the criteria of minimal Root Mean Square Error of Prediction of Cross Validation (RMSEPcv) and maximal coefficient of determination (R2cv) and Residual Prediction Deviation (RPD), the SVMR models with the first derivative pretreatment provided the most accurate prediction for As (R2cv) = 0.89, RMSEPcv = 1.89, RPD = 2.63). Less accurate, but acceptable prediction for screening purposes for Cd and Cu (0.66 ˂ R2cv) ˂ 0.81, RMSEPcv = 0.0.8 and 4.08 respectively, 2.0 ˂ RPD ˂ 2.5) were obtained. The PLSR model for predicting Mn (R2cv) = 0.44, RMSEPcv = 116.43, RPD = 1.45) presented an inadequate model. Overall, SVMR models for the Vis-NIR spectra could be used indirectly for an accurate assessment of PTEs’ concentrations.
Url:
DOI: 10.1371/journal.pone.0117457
PubMed: 25692671
PubMed Central: 4333826
Affiliations:
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University of Life Science, Kamýcká 129, 165 21- Suchdol, Praha 6- Prague, Czech Republic</addr-line></nlm:aff><country xml:lang="fr">République tchèque</country><wicri:regionArea>Department of Soil Science and Soil Protection, Faculty of Agrobiology, Food and Natural Resources, Czech University of Life Science, Kamýcká 129, 165 21- Suchdol, Praha 6- Prague</wicri:regionArea><wicri:noRegion>Praha 6- Prague</wicri:noRegion></affiliation></author><author><name sortKey="Boruvka, Lubos" sort="Boruvka, Lubos" uniqKey="Boruvka L" first="Luboš" last="Borůvka">Luboš Borůvka</name><affiliation wicri:level="1"><nlm:aff id="aff001"><addr-line>Department of Soil Science and Soil Protection, Faculty of Agrobiology, Food and Natural Resources, Czech University of Life Science, Kamýcká 129, 165 21- Suchdol, Praha 6- Prague, Czech Republic</addr-line></nlm:aff><country xml:lang="fr">République tchèque</country><wicri:regionArea>Department of Soil Science and Soil Protection, Faculty of Agrobiology, Food and Natural Resources, Czech University of Life Science, Kamýcká 129, 165 21- Suchdol, Praha 6- Prague</wicri:regionArea><wicri:noRegion>Praha 6- Prague</wicri:noRegion></affiliation></author><author><name sortKey="Vasat, Radim" sort="Vasat, Radim" uniqKey="Vasat R" first="Radim" last="Vašát">Radim Vašát</name><affiliation wicri:level="1"><nlm:aff id="aff001"><addr-line>Department of Soil Science and Soil Protection, Faculty of Agrobiology, Food and Natural Resources, Czech University of Life Science, Kamýcká 129, 165 21- Suchdol, Praha 6- Prague, Czech Republic</addr-line></nlm:aff><country xml:lang="fr">République tchèque</country><wicri:regionArea>Department of Soil Science and Soil Protection, Faculty of Agrobiology, Food and Natural Resources, Czech University of Life Science, Kamýcká 129, 165 21- Suchdol, Praha 6- Prague</wicri:regionArea><wicri:noRegion>Praha 6- Prague</wicri:noRegion></affiliation></author><author><name sortKey="Saberioon, Mohammadmehdi" sort="Saberioon, Mohammadmehdi" uniqKey="Saberioon M" first="Mohammadmehdi" last="Saberioon">Mohammadmehdi Saberioon</name><affiliation wicri:level="1"><nlm:aff id="aff002"><addr-line>Laboratory of Image and Signal Processing, Institute of Complex Systems, Faculty of Fisheries and Protection of Waters, University of South Bohemia in České Budějovice, Zámek 136 37 333- Nové Hrady, Czech Republic</addr-line></nlm:aff><country xml:lang="fr">République tchèque</country><wicri:regionArea>Laboratory of Image and Signal Processing, Institute of Complex Systems, Faculty of Fisheries and Protection of Waters, University of South Bohemia in České Budějovice, Zámek 136 37 333- Nové Hrady</wicri:regionArea><wicri:noRegion>Zámek 136 37 333- Nové Hrady</wicri:noRegion></affiliation></author><author><name sortKey="Klement, Ales" sort="Klement, Ales" uniqKey="Klement A" first="Aleš" last="Klement">Aleš Klement</name><affiliation wicri:level="1"><nlm:aff id="aff001"><addr-line>Department of Soil Science and Soil Protection, Faculty of Agrobiology, Food and Natural Resources, Czech University of Life Science, Kamýcká 129, 165 21- Suchdol, Praha 6- Prague, Czech Republic</addr-line></nlm:aff><country xml:lang="fr">République tchèque</country><wicri:regionArea>Department of Soil Science and Soil Protection, Faculty of Agrobiology, Food and Natural Resources, Czech University of Life Science, Kamýcká 129, 165 21- Suchdol, Praha 6- Prague</wicri:regionArea><wicri:noRegion>Praha 6- Prague</wicri:noRegion></affiliation></author><author><name sortKey="Kratina, Josef" sort="Kratina, Josef" uniqKey="Kratina J" first="Josef" last="Kratina">Josef Kratina</name><affiliation wicri:level="1"><nlm:aff id="aff001"><addr-line>Department of Soil Science and Soil Protection, Faculty of Agrobiology, Food and Natural Resources, Czech University of Life Science, Kamýcká 129, 165 21- Suchdol, Praha 6- Prague, Czech Republic</addr-line></nlm:aff><country xml:lang="fr">République tchèque</country><wicri:regionArea>Department of Soil Science and Soil Protection, Faculty of Agrobiology, Food and Natural Resources, Czech University of Life Science, Kamýcká 129, 165 21- Suchdol, Praha 6- Prague</wicri:regionArea><wicri:noRegion>Praha 6- Prague</wicri:noRegion></affiliation></author><author><name sortKey="Tejneck, Vaclav" sort="Tejneck, Vaclav" uniqKey="Tejneck V" first="Václav" last="Tejneck">Václav Tejneck</name><affiliation wicri:level="1"><nlm:aff id="aff001"><addr-line>Department of Soil Science and Soil Protection, Faculty of Agrobiology, Food and Natural Resources, Czech University of Life Science, Kamýcká 129, 165 21- Suchdol, Praha 6- Prague, Czech Republic</addr-line></nlm:aff><country xml:lang="fr">République tchèque</country><wicri:regionArea>Department of Soil Science and Soil Protection, Faculty of Agrobiology, Food and Natural Resources, Czech University of Life Science, Kamýcká 129, 165 21- Suchdol, Praha 6- Prague</wicri:regionArea><wicri:noRegion>Praha 6- Prague</wicri:noRegion></affiliation></author><author><name sortKey="Drabek, Ond Ej" sort="Drabek, Ond Ej" uniqKey="Drabek O" first="Ond Ej" last="Drábek">Ond Ej Drábek</name><affiliation wicri:level="1"><nlm:aff id="aff001"><addr-line>Department of Soil Science and Soil Protection, Faculty of Agrobiology, Food and Natural Resources, Czech University of Life Science, Kamýcká 129, 165 21- Suchdol, Praha 6- Prague, Czech Republic</addr-line></nlm:aff><country xml:lang="fr">République tchèque</country><wicri:regionArea>Department of Soil Science and Soil Protection, Faculty of Agrobiology, Food and Natural Resources, Czech University of Life Science, Kamýcká 129, 165 21- Suchdol, Praha 6- Prague</wicri:regionArea><wicri:noRegion>Praha 6- Prague</wicri:noRegion></affiliation></author></analytic><series><title level="j">PLoS ONE</title><idno type="eISSN">1932-6203</idno><imprint><date when="2015">2015</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en"><p>In order to monitor Potentially Toxic Elements (PTEs) in anthropogenic soils on brown coal mining dumpsites, a large number of samples and cumbersome, time-consuming laboratory measurements are required. Due to its rapidity, convenience and accuracy, reflectance spectroscopy within the Visible-Near Infrared (Vis-NIR) region has been used to predict soil constituents. This study evaluated the suitability of Vis-NIR (350–2500 nm) reflectance spectroscopy for predicting PTEs concentration, using samples collected on large brown coal mining dumpsites in the Czech Republic. Partial Least Square Regression (PLSR) and Support Vector Machine Regression (SVMR) with cross-validation were used to relate PTEs data to the reflectance spectral data by applying different preprocessing strategies. According to the criteria of minimal Root Mean Square Error of Prediction of Cross Validation (RMSEP<sub>cv</sub>) and maximal coefficient of determination (R<sup>2</sup><sub>cv</sub>) and Residual Prediction Deviation (RPD), the SVMR models with the first derivative pretreatment provided the most accurate prediction for As (R<sup>2</sup><sub>cv</sub>) = 0.89, RMSEP<sub>cv</sub> = 1.89, RPD = 2.63). Less accurate, but acceptable prediction for screening purposes for Cd and Cu (0.66 ˂ R<sup>2</sup><sub>cv</sub>) ˂ 0.81, RMSEP<sub>cv</sub> = 0.0.8 and 4.08 respectively, 2.0 ˂ RPD ˂ 2.5) were obtained. The PLSR model for predicting Mn (R<sup>2</sup><sub>cv</sub>) = 0.44, RMSEP<sub>cv</sub> = 116.43, RPD = 1.45) presented an inadequate model. Overall, SVMR models for the Vis-NIR spectra could be used indirectly for an accurate assessment of PTEs’ concentrations.</p></div></front><back><div1 type="bibliography"><listBibl><biblStruct><analytic><author><name sortKey="Li, Ms" uniqKey="Li M">MS Li</name></author></analytic></biblStruct><biblStruct><analytic><author><name sortKey="Strudl, M" uniqKey="Strudl M">M Strudl</name></author><author><name sortKey="Boruvka, L" uniqKey="Boruvka L">L Boruvka</name></author><author><name sortKey="Dimitrovsky, K" uniqKey="Dimitrovsky K">K Dimitrovsky</name></author><author><name sortKey="Kozak, J" uniqKey="Kozak J">J Kozak</name></author></analytic></biblStruct><biblStruct><analytic><author><name sortKey="Wu, Y" uniqKey="Wu Y">Y Wu</name></author><author><name sortKey="Chen, J" uniqKey="Chen J">J Chen</name></author><author><name sortKey="Wu, X" uniqKey="Wu X">X Wu</name></author><author><name sortKey="Tian, Q" uniqKey="Tian Q">Q Tian</name></author><author><name sortKey="Ji, J" uniqKey="Ji 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uniqKey="Stevens A">A Stevens</name></author><author><name sortKey="Udelhoven, T" uniqKey="Udelhoven T">T Udelhoven</name></author><author><name sortKey="Denis, A" uniqKey="Denis A">A Denis</name></author><author><name sortKey="Tychon, B" uniqKey="Tychon B">B Tychon</name></author><author><name sortKey="Lioy, R" uniqKey="Lioy R">R Lioy</name></author></analytic></biblStruct></listBibl></div1></back></TEI><affiliations><list><country><li>République tchèque</li></country></list><tree><country name="République tchèque"><noRegion><name sortKey="Gholizadeh, Asa" sort="Gholizadeh, Asa" uniqKey="Gholizadeh A" first="Asa" last="Gholizadeh">Asa Gholizadeh</name></noRegion><name sortKey="Boruvka, Lubos" sort="Boruvka, Lubos" uniqKey="Boruvka L" first="Luboš" last="Borůvka">Luboš Borůvka</name><name sortKey="Drabek, Ond Ej" sort="Drabek, Ond Ej" uniqKey="Drabek O" first="Ond Ej" last="Drábek">Ond Ej Drábek</name><name sortKey="Klement, Ales" sort="Klement, Ales" uniqKey="Klement A" first="Aleš" last="Klement">Aleš Klement</name><name sortKey="Kratina, Josef" sort="Kratina, Josef" uniqKey="Kratina J" first="Josef" last="Kratina">Josef Kratina</name><name sortKey="Saberioon, Mohammadmehdi" sort="Saberioon, Mohammadmehdi" uniqKey="Saberioon M" first="Mohammadmehdi" last="Saberioon">Mohammadmehdi Saberioon</name><name sortKey="Tejneck, Vaclav" sort="Tejneck, Vaclav" uniqKey="Tejneck V" first="Václav" last="Tejneck">Václav Tejneck</name><name sortKey="Vasat, Radim" sort="Vasat, Radim" uniqKey="Vasat R" first="Radim" last="Vašát">Radim Vašát</name></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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